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ChemicalBook CAS DataBase List Methyl 2-aminopyridine-4-carboxylate
6937-03-7

Methyl 2-aminopyridine-4-carboxylate synthesis

14synthesis methods
-

Yield:6937-03-7 93.9%

Reaction Conditions:

Stage #1:2-Amino-4-methylpyridine with nitric acid in water at 40; for 4 h;
Stage #2:methanol; pH=9 for 2 h;Reflux;Temperature;pH-value;

Steps:

3 Synthesis of 2-aminopyridine-4-carboxylic acid methyl ester
(2) 2-Amino-4-methylpyridine was mixed with water,Heat to 40°C, add Fe-Mn-Mo-TiO catalyst,After stirring, dilute nitric acid is added dropwise.Stir the reaction for 4h,After falling to room temperature,filter,The filtrate was adjusted to pH 9,After adding methanol,After heating and refluxing for 2h,Vacuum distillation to remove methanolMultiple extractions with dichloromethane,Combine the organic phase,Distillation under reduced pressure to remove the dichloromethane,Preparation of 2-aminopyridine-4-carboxylic acid methyl ester.Fe(NO3)3, in step (1)MnCl2,The molar ratio of molybdenum was 4:7:1, the mass ratio of Fe(NO3)3 to nano-TiO2 particles was 1:1, and the molar ratio of NaOH and Na2CO3 was 4:1.In step (2), the mass ratio of 2-amino-4-methylpyridine to Fe-Mn-Mo-TiO catalyst is 11:2.The mass concentration of nitric acid was 30%, the molar ratio of 2-amino-4-methylpyridine to nitric acid was 1:1.5, and the molar ratio of 2-amino-4-methylpyridine to methanol was 1:1.The methyl 2-aminopyridine-4-carboxylate was prepared with a purity of 99.4% and a yield of 93.9%.

References:

Suzhou Aitike Pharmaceutical Chemical Co., Ltd.;Hu Haiwei CN107868040, 2018, A Location in patent:Paragraph 0021-0031; 0032-0038; 0042-0045; 0049-0051

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