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ChemicalBook CAS DataBase List TERT-BUTYL 3-OXO-2,8-DIAZASPIRO[4.5]DECANE-8-CARBOXYLATE
169206-67-1

TERT-BUTYL 3-OXO-2,8-DIAZASPIRO[4.5]DECANE-8-CARBOXYLATE synthesis

7synthesis methods
-

Yield:169206-67-1 86%

Reaction Conditions:

with hydrogen;nickel in ethanol under 760.051 Torr;

Steps:

50.3
To a solution of 4-methoxycarbonylmethyl-4-nitromethyl-piperidine-1-carboxylic acid tert-butyl ester (1.0 g, 3.2 mmol) in ethanol (10 mL) was added Raney Ni (1 g). The resulting suspension was hydrogenated at 1 atm overnight. The mixture was filtered through Celite and evaporated in vacuo. The residue was purified with silica gel column chromatography (10% methanol in dichloromethane) to give the desired lactam (694 mg, 86%). 1H NMR (400 MHz, CD3OD) δ 3.54-3.48 (m, 2H), 3.37-3.32 (m, 2H), 3.23 (s, 2H), 2.26 (s, 2H), 1.62-1.59 (m, 4H), 1.45 (s, 9H).

References:

Cumbre Inc. US2006/19985, 2006, A1 Location in patent:Page/Page column 55

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