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CAS No. : | 5466-43-3 | MDL No. : | MFCD09750204 |
Formula : | C7H6Cl2N2 | Boiling Point : | No data available |
Linear Structure Formula : | - | InChI Key : | GDHHAOFBLGZCMI-UHFFFAOYSA-N |
M.W : | 189.04 | Pubchem ID : | 231331 |
Synonyms : |
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Signal Word: | Warning | Class: | |
Precautionary Statements: | P305+P351+P338 | UN#: | |
Hazard Statements: | H302-H319 | Packing Group: | |
GHS Pictogram: |
* All experimental methods are cited from the reference, please refer to the original source for details. We do not guarantee the accuracy of the content in the reference.
Yield | Reaction Conditions | Operation in experiment |
---|---|---|
42% | With N-ethyl-N,N-diisopropylamine; In isopropyl alcohol; at 100℃; for 16h; | Synthesis of 2-chloro-N-(5-isopropyl-1H-pyrazol-3-yl)-6,7-dihydro-5H-cyclopenta[d]pyrimidin-4-amine, Compound (iii) To a solution of 2,4-dichloro-6,7-dihydro-5H-cyclopenta[d]pyrimidine, Compound (i) (8 g, 42 mmol) in isopropanol (100 mL) was added N,N-diisopropylethyl amine (8.67 g, 67 mmol) followed by <strong>[56367-24-9]5-isopropyl-1H-pyrazol-3-amine</strong>, Compound (ii) (5.89 g, 47 mmol). The reaction mixture was heated to reflux at 100 C. for 16 h. The reaction mixture was cooled to RT. The precipitated product was filtered and washed with hexane to afford 2-chloro-N-(5-isopropyl-1H-pyrazol-3-yl)-6,7-dihydro-5H-cyclopenta[d]pyrimidin-4-amine, Compound (iii) (5 g, 42%). 1H NMR (400 MHz, DMSO-d6) δ (ppm): 1.22 (d, 6H), 1.96-2.07 (m, 2H), 2.70-2.81 (m, 4H), 2.88-3.01 (m, 1H), 6.38 (s, 1H), 9.60 (s, 1H), 12.11 (brs, 1H). |
34% | With triethylamine; In ethanol; for 48h;Reflux; | The compound of example 2 (3.17 mmol) and 5-isopropyl- 1 H-pyrazol-3-amine (3.17 mmol) were refluxed in ethanol in the presence of triethylamine (15.87 mmol) for 48 h. The resulting reaction mixture was cooled and filtered to obtain the title compound. Yield: 34 %; ‘H NMR(DMSO-d6, 300 MHz): 12.16 (s, 1H), 9.61 (s, 1H), 6.37 (s, 1H), 2.94 (m, 1H), 2.74 (m, 4H),2.00 (m, 2.00), 1.23 (d, 6H); HRMS (+ve): 278.1180. |
Yield | Reaction Conditions | Operation in experiment |
---|---|---|
39% | In 1-methyl-pyrrolidin-2-one; at 80℃; | 2-(4-Aminophenyl)acetic acid tert-butyl ester (2.00 g, 9.66 mmol) and 2,4-dichloro-6,7-dihydro-5H- cyclopenta[d]pyrimidine (1.74 g, 9.20 mmol) in NMP (46 ml) were stirred overnight at 80C. After cooling to room temperature, ethyl acetate (200 ml) was added, the mixture was washed with water and dried with magnesium sulfate. The solvent was distilled off and the residue stirred with methanol and hexane. The solid was filtered and dried under vacuum. Brown solid. Yield: 1.3 g (39% of theoretical). |
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